Within the present examine, diamond-like carbon (DLC) was synthesized by pulsed laser deposition (PLD) in a vacuum at room temperature, specializing in Ni-dopant focus and association of Ni strips in each parallel and transverse positions. The morphology and structural properties of Ni-DLC movies have been analyzed by Raman spectroscopy, atomic power microscopy (AFM) evaluation, cross-section evaluation, energy-dispersive X-ray spectroscopy (EDS), X-ray photoelectron spectroscopy (XPS), contact angle (CA), and nanoindentation take a look at. AFM photos exhibit the brand new shapes of Ni-DLC skinny movies, named conic and nano-mushroom particles. The Raman spectra of Ni-DLC movies present that the calculated intensities D-line to G-line ratio experiences a lower with growing Ni dopants within the transverse association whereas the parallel association represents a unique development. The stoichiometry of Ni-DLC skinny movies has been reported from the cross-section of skinny movies. It’s also noticed from the measured CA that the hydrophilic properties of Ni-DLCs improve within the transverse association. Low nickel content material in diamond-like carbon matrix exhibited the dominance of diamond section and good mechanical properties have been discovered.